Around 2003, tungsten bronze (TB) crystal materials were widely used in laser frequency doubling, electro-optical modulation, optical information processing, superconductivity, humidity sensors, Solid fuel cells and other technical fields. In 2006, Koichi Tatsumi et al. synthesized tungsten bronze in which M is metal elements such as Sn, Pb, Cu, Sb and Zn. W in tungsten bronze exists in mixed valence states such as W6 +, W5+ and W4 +, so that the overall charge of the compound balance. The tunnel structure and this special valence state make it have excellent properties, such as electronic and ionic conductivity, superconductivity, optical properties, etc., and its applications in secondary batteries, electrochromic and chemical sensors have attracted extensive attention. research interests.
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